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HOME > PAST ISSUE > March-April 2006 > Article Detail

FEATURE ARTICLE

Filaments of Light

Pulsed terawatt lasers create some surprising effects when shone through the air—including the channeling of light

Jérôme Kasparian

Bug Zapper Extraordinaire

The fact that the Kerr effect can transform a high-power infrared laser into a remote source of white light opens the door to a number of exciting applications. For example, the tendency for some of the light to be reflected backward suggests that we could create an artificial "guide star" for use in adjusting astronomical telescopes equipped with adaptive optics. But there are other nonlinear optical effects of the Teramobile laser that can be exploited as well. One is something called multiphoton fluorescence.

In normal fluorescence, a substance, say the phosphor powder that coats the inside of a fluorescent lamp, absorbs high-energy photons (typically in the ultraviolet) and releases lower-energy photons (having, usually, visible-light wavelengths). In multiphoton fluorescence, two or more low-energy photons are absorbed simultaneously, raising an electron's energy level enough to allow a single high-energy photon to be given off when the electron returns to its original state. But because the chance of an atom absorbing two photons at once is quite low, light of very high intensity (that is, containing a very large number of photons) is needed. The pulsed Teramobile laser provides just such light, which proves a great boon for remotely sensing certain compounds using the phenomenon of multiphoton fluorescence.

In a 2002 experiment, my colleagues and I showed that the Teramobile beam and detection apparatus could sense biological aerosols at a distance. The motivation was to be able to map a cloud, say, of bacteria (perhaps given off during some industrial mishap or even a biological attack) and to identify potentially pathogenic agents among the various background atmospheric aerosols, among which may be more mundane organic particles such as soot or pollen.

Figure 9. In 2002, the Teramobile laser was used...Click to Enlarge Image

Our test used water droplets sized to mimic bacteria and laced with the compound riboflavin, which fluoresces at visible wavelengths when it absorbs two infrared photons, producing a characteristic spectrum in the backscattered light. The experiment, carried out on a cloud located about 45 meters from the Teramobile laser, showed that it was easy to distinguish such a plume from a cloud of pure water droplets. With refinement, this technique could, potentially, be quite sensitive. We calculated that a laser tuned to excite two-photon fluorescence in the amino acid tryptophan would boost sensitivity by a factor of 10, allowing concentrations of as little as 10 bacteria per cubic centimeter to be detected 4 kilometers away. Although lidar systems based on normal fluorescence could also be used to probe for biological agents, the laser employed would have to operate at a shorter wavelength and thus be more prone to attenuation, limiting the distance over which it could function effectively.

The ability of laser filaments to deliver high-intensity light at substantial distances also opens the door to other very interesting applications. For example, it becomes possible to conduct elemental analyses of the surfaces of metals, plastics, minerals or liquids from an appreciable distance, using a variation of a technique called laser-induced breakdown spectroscopy. For that, a powerful laser is focused on the material of interest, causing some of it to be transformed into plasma. The emission spectrum of the glowing plasma can then be analyzed, revealing the nature of the substrate, with a detection limit that can be as little as a few parts per million for some elements. This method is currently used for such applications as the identification of highly radioactive nuclear waste and for monitoring the composition of molten alloys, because the tests can be performed without having to touch the sample. Imagine being able to do such probing from a large distance away! Normally, diffraction limits the intensity of light that can be focused on a remote target. But laser filaments can deliver intensities that are higher than the ablation threshold of many types of materials, at distances of hundreds of meters or even kilometers.

Figure 10. Experiments with the Teramobile laser...Click to Enlarge Image

Another application under investigation may prove more spectacular yet—the control of lightning strikes. Lightning has always fascinated people, in part because of its unpredictable nature and destructive power—qualities that make these electrical discharges very difficult to study. Investigators from Electricité de France and CEA partially overcame those obstacles in the 1970s, when they developed a technique to trigger lightning on command using small rockets trailing thin wires. If shot upward at the right moment, the rockets and the wires they unspooled behind them served to initiate and channel the flow of electric current.

One outgrowth of this work was the idea of using a high-intensity laser to ionize air along the beam, thus forming a conducting channel of plasma that could replace the rocket-hoisted wires. The first attempts, mounted in the 1970s and '80s, used lasers that produced nanosecond-long pulses. Those experiments were unsuccessful, however, because the plasma created by such lasers is largely opaque, which keeps the beam from extending a conductive path very far. But recently this field of research has seen renewed interest, because lasers can now provide higher intensities in shorter pulses, thereby avoiding the severe absorption that would otherwise occur. In particular, the team of Henri Pépin (Institut national de la recherche scientifique) and Hubert P. Mercure (Hydro-Québec) in Montreal have obtained quite promising results, using pulsed lasers to trigger and guide high-voltage discharges over several meters in the laboratory.

Spectacular experiments with the Teramobile system, installed in a high-voltage facility at the Technische Universität Berlin, showed that laser filaments can trigger and guide electric discharges over distances exceeding 4 meters. Moreover, the breakdown voltage is typically reduced by 30 percent. My colleagues and I have also shown that rain (or rather simulated rain) does not prevent the laser filaments from triggering these huge sparks. Research now focuses on the possibility of extending the lifetime of the plasma and increasing the length over which it is able to guide a discharge. Although the control of real lightning remains science fiction for the moment, recent progress in laser technology has brought this three-decade-old dream much closer to reality.

Over the past few years, the capabilities of terawatt-class lasers have improved markedly, while size and cost have come down. At the same time, physicists have made great strides in understanding the non-linear propagation of these high-power laser pulses in air. The rapidity of this progress suggests that Teramobile-type lasers, or systems like it, might soon be used widely, not just by scientists in the course of their research but for any number of military, commercial or public-safety applications.

Bibliography

  • Kasparian, J, M. Rodriguez, G. Méjean, J. Yu, E. Salmon, H. Wille, R. Bourayou, S. Frey, Y.-B. André, A. Mysyrowicz, R. Sauerbrey, J.-P. Wolf and L. Wöste. 2003. White-light filaments for atmospheric analysis. Science 301:61-64.
  • Wille, H., M. Rodriguez, J. Kasparian, D. Mondelain, J. Yu, A. Mysyrowicz, R. Sauerbrey, J.-P. Wolf and L. Wöste. 2002. Teramobile: A mobile femtosecond-terawatt laser and detection system. European Physical Journal—Applied Physics 20:183-190.
  • Kasparian, J, S. Frey, G. Méjean, E. Salmon, J. Yu, J.-P. Wolf, R. Bourayou, J.-C. Luderer, M. Rodriguez, H. Wille and L. Wöste. 2005. Femtosecond white-light lidar. In Laser Remote Sensing. Ed. T. Fujii and T. Fukuchi. New York: Marcel Dekker.




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